Van der Waals Nanowires with Continuously Variable Interlayer Twist and Twist Homojunctions
Abstract
Moiré patterns at van der Waals interfaces between twisted 2D crystals give rise to distinct optoelectronic excitations, as well as, narrowly dispersive bands responsible for correlated electron phenomena. Contrasting with the conventional, mechanically stacked planar twist moirés, recent work shows twisted van der Waals interfaces spontaneously formed in nanowires of layered crystals, where Eshelby twist due to axial screw dislocations stabilizes a chiral structure with small interlayer rotation. Here, the realization of tunable twist in germanium(II) sulfide (GeS) van der Waals nanowires is reported. Tapered nanowires host continuously variable interlayer twist. Homojunctions between dislocated (chiral) and defect‐free (achiral) segments are obtained by triggering the emission of axial dislocations during growth. Measurements across such junctions, implemented here using local absorption and luminescence spectroscopy, provide a convenient tool for detecting twist effects. The results identify a versatile system for 3D twistronics, probing moiré physics, and for realizing moiré architectures without equivalent in planar systems.
Document Details
- Document Type
- Pub Defense Publication
- Publication Date
- Dec 03, 2020
- Source ID
- 10.1002/adfm.202006412
Entities
People
- Eli Sutter
- Juan‐carlos Idrobo
- Peter Sutter
Organizations
- Battelle Memorial Institute
- Division of Materials Research
- National Science Foundation
- Oak Ridge National Laboratory
- Office of Naval Research
- United States Department of Energy
- United States Navy
- University of Nebraska–Lincoln