An Electrochemical Gelation Method for Patterning Conductive PEDOT:PSS Hydrogels

Abstract

Due to their high water content and macroscopic connectivity, hydrogels made from the conducting polymer PEDOT:PSS are a promising platform from which to fabricate a wide range of porous conductive materials that are increasingly of interest in applications as varied as bioelectronics, regenerative medicine, and energy storage. Despite the promising properties of PEDOT:PSS‐based porous materials, the ability to pattern PEDOT:PSS hydrogels is still required to enable their integration with multifunctional and multichannel electronic devices. In this work, a novel electrochemical gelation (“electrogelation”) method is presented for rapidly patterning PEDOT:PSS hydrogels on any conductive template, including curved and 3D surfaces. High spatial resolution is achieved through use of a sacrificial metal layer to generate the hydrogel pattern, thereby enabling high‐performance conducting hydrogels and aerogels with desirable material properties to be introduced into increasingly complex device architectures.

Document Details

Document Type
Pub Defense Publication
Publication Date
Aug 15, 2019
Source ID
10.1002/adma.201902869

Entities

People

  • David G. Mackanic
  • Helen Tran
  • Kathy Liu
  • Levent Beker
  • Minah Lee
  • Vivian Rachel Feig
  • Zhenan Bao
  • Zhuojun Huang

Organizations

  • Intelligence Community Postdoctoral Research Fellowship Program
  • Korea Institute of Science and Technology
  • Koç University
  • National Science Foundation
  • Oak Ridge Institute for Science and Education
  • Office of the Director of National Intelligence
  • Stanford University
  • United States Department of Defense
  • United States Department of Energy

Tags

Fields of Study

  • Materials science

Readers

  • Nanocomposite Materials Science

Technology Areas

  • Biotechnology
  • Microelectronics