Gas Separations using Nanoporous Atomically Thin Membranes: Recent Theoretical, Simulation, and Experimental Advances

Abstract

Porous graphene and other atomically thin 2D materials are regarded as highly promising membrane materials for high‐performance gas separations due to their atomic thickness, large‐scale synthesizability, excellent mechanical strength, and chemical stability. When these atomically thin materials contain a high areal density of gas‐sieving nanoscale pores, they can exhibit both high gas permeances and high selectivities, which is beneficial for reducing the cost of gas‐separation processes. Here, recent modeling and experimental advances in nanoporous atomically thin membranes for gas separations is discussed. The major challenges involved, including controlling pore size distributions, scaling up the membrane area, and matching theory with experimental results, are also highlighted. Finally, important future directions are proposed for real gas‐separation applications of nanoporous atomically thin membranes.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jun 19, 2022
Source ID
10.1002/adma.202201472

Entities

People

  • Daniel Blankschtein
  • Guangwei He
  • Michael Strano
  • Rahul Prasanna Misra
  • Sylvia Xin Li
  • Zhe Yuan

Organizations

  • Army Research Office
  • Massachusetts Institute of Technology
  • National Science Foundation
  • Office of Basic Energy Sciences
  • Office of Science
  • Swiss National Science Foundation
  • United States Army Research Laboratory
  • United States Department of Energy

Tags

Fields of Study

  • Chemistry

Readers

  • Combustion and Flow Dynamics.
  • Nanocomposite Materials Science

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene