4D Printing of Freestanding Liquid Crystal Elastomers via Hybrid Additive Manufacturing

Abstract

Liquid crystal elastomers (LCE) are appealing candidates among active materials for 4D printing, due to their reversible, programmable and rapid actuation capabilities. Recent progress has been made on direct ink writing (DIW) or Digital Light Processing (DLP) to print LCEs with certain actuation. However, it remains a challenge to achieve complicated structures, such as spatial lattices with large actuation, due to the limitation of printing LCEs on the build platform or the previous layer. Herein, a novel method to 4D print freestanding LCEs on‐the‐fly by using laser‐assisted DIW with an actuation strain up to −40% is proposed. This process is further hybridized with the DLP method for optional structural or removable supports to create active 3D architectures in a one‐step additive process. Various objects, including hybrid active lattices, active tensegrity, an actuator with tunable stability, and 3D spatial LCE lattices, can be additively fabricated. The combination of DIW‐printed functionally freestanding LCEs with the DLP‐printed supporting structures thus provides new design freedom and fabrication capability for applications including soft robotics, smart structures, active metamaterials, and smart wearable devices.

Document Details

Document Type
Pub Defense Publication
Publication Date
Aug 29, 2022
Source ID
10.1002/adma.202204890

Entities

People

  • Frédéric Demoly
  • H. Jerry Qi
  • Kun Zhou
  • Liang Yue
  • Ruike Renee Zhao
  • S. Macrae Montgomery
  • Shuai Wu
  • Xiaohao Sun
  • Xirui Peng

Organizations

  • Air Force Office of Scientific Research
  • Georgia Tech
  • Nanyang Technological University
  • National Science Foundation
  • Stanford University

Tags

Readers

  • Nanocomposite Materials Science
  • Nanofabrication and Microfabrication.
  • Robotics and Automation.

Technology Areas

  • AI & ML
  • Autonomy
  • Directed Energy
  • Microelectronics
  • Microelectronics - Graphene
  • Microelectronics - Microelectromechanical Systems