Macroscopic Self‐Assembly and Optical Characterization of Nanoparticle–Ligand Metamaterials

Abstract

A self‐assembled metamaterial exhibiting a positive near‐zero index of refraction at visible wavelengths is demonstrated. The metamaterial consists of thiolene‐functionalized gold nanospheres self‐assembled into macroscopic, crosslinked, monolayers. By measuring the real and imaginary parts of the phase shift of light transmitted through the self‐assembled films the effective index of refraction is determined as a function of wavelength. These findings may pave a way to simply and efficiently self‐assemble and optically characterize multifunctional, multilayer nanoparticle–ligand metamaterials.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jan 01, 2013
Source ID
10.1002/adom.201200039

Entities

People

  • Banahalli R. Ratna
  • Jake Fontana
  • Jawad Naciri
  • Ronald Rendell

Organizations

  • Office of Naval Research
  • United States Naval Research Laboratory

Tags

Fields of Study

  • Physics

Readers

  • Electrochemical Surface Science
  • Electromagnetic Wave Scattering and Antenna Radiation Engineering
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Biotechnology
  • Microelectronics