Conjugated Polymer Blends for High Contrast Black‐to‐Transmissive Electrochromism

Abstract

Next‐generation electrochromic technologies, such as dimmable fenestration, eyewear integrated displays, and optical shutters require materials that reversibly transition between highly transmissive and broadly absorbing achromatic states, often with minimal intermediate coloration. In this work, it is shown how the properties of dioxythiophene‐based electrochromic polymers (ECPs) can be leveraged through straightforward color mixing to yield high‐contrast, black‐to‐transmissive materials with low driving voltages (C*ab < 5) and integrated optical contrast exceeding 40% across the entire visible spectrum (380–780 nm). By incorporating different high‐gap and dual‐band absorbing ECPs, subtle control is demonstrated over both the extreme and intermediate coloration of the blends. This work showcases how solution coprocessing of ECPs can be used to access highly targeted achromatic hues while also enabling fine‐tuned neutral optical transition between black and transmissive states.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jul 01, 2018
Source ID
10.1002/adom.201800594

Entities

People

  • Anna M Österholm
  • Dwanleen Eric Shen
  • Dylan T Christiansen
  • John R Reynolds
  • Lisa R Savagian
  • Michael Kuepfert

Organizations

  • Air Force Office of Scientific Research
  • BASF
  • Georgia Tech
  • National Science Foundation

Tags

Fields of Study

  • Physics

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Human-Computer Interaction (HCI).
  • Optical Physics and Photonics.