A Solid Oxide Fuel Cell Runs on Hydrocarbon Fuels with Exceptional Durability and Power Output

Abstract

Solid oxide fuel cells (SOFCs) that can operate on hydrocarbon fuels offer an efficient and cost‐effective solution for electricity generation. However, broader commercialization of SOFCs is hindered by inadequate performance and limited durability due to the sluggish hydrocarbon reforming/oxidation kinetics and coking on the SOFC anode. Here it has been reported that these findings in design, synthesis, and characterization of a novel anode catalyst Ba(Zr0.8Y0.2)0.9(Ni0.5Ru0.5)0.1O3‐δ (BZYNR) that overcomes the problems, enabling direct utilization of nearly dry hydrocarbon fuels (e.g., methane, ethanol, and iso‐octane with only 3 vol% H2O) with exceptional power output for over 1000 h on both button cells and tubular cells. The outstanding performance of BZYNR is attributed to the high activity of hydrocarbon reforming and the accelerated water‐mediated carbon cleaning process on Ni‐based SOFC anode.

Document Details

Document Type
Pub Defense Publication
Publication Date
Oct 27, 2022
Source ID
10.1002/aenm.202202928

Entities

People

  • Drew Spradling
  • Gyutae Nam
  • Jie Hou
  • Meilin Liu
  • Nicholas Kane
  • Tongtong Li
  • Weilin Zhang
  • Weining Wang
  • Xueyu Hu
  • Yong Ding
  • Yoojin Ahn
  • Yucun Zhou
  • Zheyu Luo
  • Zhijun Liu

Organizations

  • Army Research Office
  • Georgia Tech

Tags

Fields of Study

  • Materials science

Readers

  • Nanocomposite Materials Science
  • Petroleum Engineering
  • Systems Analysis and Design

Technology Areas

  • Biotechnology