Semiconducting Copolymers with Naphthalene Imide/Amide π‐Conjugated Units: Synthesis, Crystallography, and Systematic Structure‐Property‐Mobility Correlations

Abstract

In a series of n‐type semiconducting naphthalene tetracarboxydiimide (NDI)‐dithiophene (T2) copolymers, structural and electronic properties trends are systematically evaluated as the number of NDI carbonyl groups is reduced from 4 in NDI to 3 in NBL (1‐amino‐4,5‐8‐naphthalene‐tricarboxylic acid‐1,8‐lactam‐4,5‐imide) to 2 in NBA (naphthalene‐bis(4,8‐diamino‐1,5‐dicarboxyl)‐amide). As the NDI‐T2 backbone torsional angle falls the LUMO energy rises. However, the thienyl attachment regiochemistry also plays an important role in less symmetric NBL and NBA. Electron mobility is greatest for N2200 (0.17 cm2 V−1 s−1) followed by PNBL‐3,8‐T2 and PNBA‐2,6‐T2 (0.11 cm2 V−1 s−1), 0.02 cm2 V−1 s−1 in PNBL‐4,8‐T2, and negligible in PNBA‐3,7‐T2. Charge transport reflects a delicate balance between electronic backbone communication (optimum for N2200 and PNBL‐4,8‐T2), backbone planarity (optimum for PNBA‐2,6‐T2 and PNBL‐3,8‐T2), LUMO energy (optimum for N2200), π–π stacking distance (optimum for PNBA‐2,6‐T2), and film crystallinity (optimum for PNBA‐2,6‐T2 and N2200). These results offer generalizable insight into semiconducting copolymer design.

Document Details

Document Type
Pub Defense Publication
Publication Date
Aug 19, 2022
Source ID
10.1002/ange.202208201

Entities

People

  • Antonio Facchetti
  • Jianglin Wu
  • Shirong Lu
  • Tobin J. Marks
  • Yao Chen

Organizations

  • Air Force Research Laboratory
  • Argonne National Laboratory
  • Chongqing Institute of Green and Intelligent Technology
  • National Institute of Standards and Technology
  • National Natural Science Foundation of China
  • National Science Foundation
  • Northwestern University
  • Office of Basic Energy Sciences

Tags

Readers

  • Polymer Science and Technology
  • Solar Photovoltaics and Thermoelectric Devices.

Technology Areas

  • Microelectronics