Fully C/N‐Polynitro‐Functionalized 2,2′‐Biimidazole Derivatives as Nitrogen‐ and Oxygen‐Rich Energetic Salts

Abstract

Through the use of a fully C/N‐functionalized imidazole‐based anion, it was possible to prepare nitrogen‐ and oxygen‐rich energetic salts. When N,N‐dinitramino imidazole was paired with nitrogen‐rich bases, versatile ionic derivatives were prepared and fully characterized by IR, and 1H, and 13C NMR spectroscopy and elemental analysis. Both experimental and theoretical evaluations show promising properties for these energetic compounds, such as high density, positive heats of formation, good oxygen balance, and acceptable stabilities. The energetic salts exhibit promising energetic performance comparable to the benchmark explosive RDX (1,3,5‐trinitrotriazacyclohexane).

Document Details

Document Type
Pub Defense Publication
Publication Date
Jan 12, 2016
Source ID
10.1002/chem.201504407

Entities

People

  • Chunlin He
  • Jean'ne Shreeve
  • Ping Yin

Organizations

  • Office of Naval Research
  • University of Idaho

Tags

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry
  • Quantum Chemistry
  • Surface Coatings Technology.