Nitramino‐ and Dinitromethyl‐Substituted 1,2,4‐Triazole Derivatives as High‐Performance Energetic Materials

Abstract

Since highly nitrated nitrogen‐rich heterocycles are important motifs in high energy density materials, extensive studies for the development of such novel molecules have been underway. A highly energetic moiety, 3‐dinitromethyl‐5‐nitramino‐1,2,4‐triazole, which consists of a triazole ring, and nitramino and dinitromethyl groups, has been designed and synthesized. By pairing with nitrogen‐rich cations, several ionic derivatives were obtained. Theoretical and experimental studies show that the hydroxylammonium salt (7) is highly dense, and has excellent detonation performance with acceptable thermal stablity and sensitivities, which are superior to those of RDX.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jun 13, 2017
Source ID
10.1002/chem.201701407

Entities

People

  • Damon A. Parrish
  • Gregory H Imler
  • Jean'ne Shreeve
  • Srinivas Dharavath
  • Yongxing Tang

Organizations

  • Defense Threat Reduction Agency
  • M J Murdock Charitable Trust
  • Office of Naval Research
  • United States Naval Research Laboratory
  • University of Idaho

Tags

Fields of Study

  • Chemistry

Readers

  • Nanocomposite Materials Science
  • Organic Chemistry
  • Rocket Propulsion.