ITP of lanthanides in microfluidic PMMA chip

Abstract

An ITP separation of eight lanthanides on a serpentine PMMA microchip with a tee junction and a 230‐mm‐long serpentine channel is described. The cover of the PMMA chip is 175 μm thick so that a C4D in microchip mode can be used to detect the lanthanides as they migrate through the microchannel. Acetate and α‐hydroxyisobutyric acid are used as complexing agents to increase the electrophoretic mobility difference between the lanthanides. Eight lanthanides are concentrated within ∼ 6 min by ITP in the microchip using 10 mM ammonium acetate at pH 4.5 as the leading electrolyte and 10 mM acetic acid at ∼ pH 3.0 as the terminating electrolyte. In addition, a 2D numerical simulation of the lanthanides undergoing ITP in the microchip is compared with experimental results using COMSOL Multiphysics v4.3a.

Document Details

Document Type
Pub Defense Publication
Publication Date
Dec 27, 2013
Source ID
10.1002/elps.201300382

Entities

People

  • Bingwen Liu
  • Cornelius F Ivory
  • Danny Bottenus
  • Sue B. Clark
  • Yongzheng Cong

Organizations

  • Defense Threat Reduction Agency
  • National Science Foundation
  • United States Department of Energy
  • United States Department of Homeland Security
  • Washington State University

Tags

Fields of Study

  • Chemistry

Readers

  • Cardiovascular Physiology
  • Integrated Circuit Design and Technology.
  • Materials Science and Engineering.