Effect of occupation of the excited states and phonon broadening on the determination of the hot carrier temperature from continuous wave photoluminescence in InGaAsP quantum well absorbers

Abstract

An InGaAsP quantum well with a type‐II band alignment is studied using continuous wave power and temperature dependent photoluminescence (PL) spectroscopy. The small energy separation between the ground state and first excited state results in significant thermal carrier redistribution and excited state occupation, particularly, with increasing excitation power and temperature. This state filling is evident as a high‐energy shoulder in the PL spectra, the same energy region where in the simplest Planck‐description the gradient is considered inversely proportional to carrier temperature. The outcome of an excited state occupation in broadening the high‐energy PL tail is to perturb the temperature extracted using this analysis; therefore, the true temperature of carriers is not properly evaluated when significant state filling occurs. In addition, broadening of the PL due to phonons at higher temperatures also distorts (or falsely increases) the non‐equilibrium “hot” carrier temperature and as such should be considered when using Planck's relation. The role of these two effects is considered and their mutual effect on the analysis of the extracted hot carrier temperature discussed. Copyright © 2017 John Wiley & Sons, Ltd.

Document Details

Document Type
Pub Defense Publication
Publication Date
Apr 17, 2017
Source ID
10.1002/pip.2890

Entities

People

  • Chase T Ellis
  • David V. Forbes
  • Hamidreza Esmaielpour
  • Ian R. Sellers
  • Joseph G Tischler
  • Louise C. Hirst
  • Matthew P. Lumb
  • Robert J. Walters
  • Vincent R. Whiteside

Organizations

  • George Washington University
  • Office of Naval Research
  • Rochester Institute of Technology
  • United States Naval Research Laboratory
  • University of Oklahoma

Tags

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Plasma Physics.
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Quantum Computing