Synthesis and characterization of alt‐copoly(carbosiloxane)s containing oligodiphenylsiloxane segments

Abstract

Novel α,ω‐divinyloligodiphenylsiloxanes (1,9‐divinyldecaphenylpentasiloxane, 1,7‐divinyloctaphenyltetrasiloxane, 1,5‐divinylhexaphenyltrisiloxane, and 1,3‐divinyltetraphenyldisiloxane) were prepared and copolymerized by Pt‐catalyzed hydrosilylation with α,ω‐dihydridopentasiloxanes. The molecular weights of the copolymers were measured with gel permeation chromatography, and their thermal properties were characterized with differential scanning calorimetry and thermogravimetric analysis. The polymers had high thermal stability in air and nitrogen. The oligomer and polymer structures were determined with 1H, 13C, 19F, and 29Si NMR and IR spectrometry. The molecular weights of the oligomers were measured with high‐resolution mass spectrometry. © 2005 Wiley Periodicals, Inc. J Polym Sci Part A: Polym Chem 43: 2155–2163, 2005

Document Details

Document Type
Pub Defense Publication
Publication Date
Apr 08, 2005
Source ID
10.1002/pola.20665

Entities

People

  • Thomas M. Gädda
  • William P. Weber

Organizations

  • Office of Naval Research

Tags

Fields of Study

  • Chemistry

Readers

  • Polymer Science and Technology

Technology Areas

  • Microelectronics