Highly soluble green‐emitting Ir(III) complexes with 9‐(6‐phenyl‐pyridin‐3‐ylmethyl)‐9H‐carbazole ligands and their application to polymer light‐emitting diodes

Abstract

Highly organic soluble Ir(III) complexes with 9‐(6‐phenyl‐pyridin‐3‐ylmethyl)‐9H‐carbazole were simply synthesized, and the solubility of the new complex was significantly improved when compared with the conventional green‐emitting Ir(ppy)3. Since a carbazole group is tethered through a nonconjugated methylene spacer, the photophysical properties of new complexes are almost identical with those of conventional Ir(ppy)3. The pure complexes were utilized to prepare electrophosphorescent polymer light‐emitting diodes (PLEDs). The device performances were observed to be relatively better or comparable with those of Ir(ppy)3 based poly(N‐vinylcarbazole) systems. The integration of rigid hole‐transporting carbazole and phosphorescent complex provides a new route to design highly efficient solution‐processable complex for electrophosphorescent PLED applications. © 2008 Wiley Periodicals, Inc. J Polym Sci Part A: Polym Chem 46: 7419–7428, 2008

Document Details

Document Type
Pub Defense Publication
Publication Date
Oct 09, 2008
Source ID
10.1002/pola.23047

Entities

People

  • Byeong‐kwon Ju
  • Chang Seop Hong
  • Dong Hoon Choi
  • Jae Il Kim
  • Min Ju Cho
  • Young Min Kim
  • Young Wook Park

Organizations

  • Air Force Office of Scientific Research
  • Ministry of Science and Technology

Tags

Fields of Study

  • Chemistry

Readers

  • Nanoscale Plasmonic Nanotechnology
  • Polymer Science and Technology
  • Semiconductor Device Technology