Determination of Thermal History by Photoluminescence of Core‐Shelled Quantum Dots Going Through Heating Events
Abstract
A kind of novel thermal history nanosensors are theoretically designed and experimentally demonstrated to permanently record thermal events. The photoluminescence (PL) spectrum of core‐shelled quantum dots (QDs) CdSe/ZnS irreversibly shifts with heating histories (temperature and duration) of thermal events. The induced PL shift of the QDs CdSe/ZnS is employed to permanently record thermal histories. We further model a kind of thermal history nanosensor based on the thermal‐induced phenomena of core‐shelled QDs to permanently record thermal histories at microscale and demonstrate to reconstruct temperature and duration of heating events simultaneously from PL spectra of the QDs. The physical mechanism of the sensors is discussed.
Document Details
- Document Type
- Pub Defense Publication
- Publication Date
- Jul 28, 2014
- Source ID
- 10.1002/ppsc.201400100
Entities
People
- Gang Chen
- Hui Wang
- Nitin Skula
- Xiaoyuan Chen
- Yalin Lu
- Yucheng Lan
- Zhifeng Ren
Organizations
- Defense Threat Reduction Agency
- Massachusetts Institute of Technology
- Morgan State University
- United States Air Force Academy
- University of Houston