Formation and Characterization of Heavy Alkali and Silver Salts of the 4‐Nitro‐pyrazolo‐(3,4‐c)‐furazan‐5‐N‐oxide Anion

Abstract

The nitration of 3‐amino‐4‐chloro‐oximidofurazan resulted in the formation of the unexpected anionic heterocycle 4‐nitro‐pyrazolo‐(3,4,c)‐furazan‐5‐N‐oxide. Various experiments such as changing the reactants, oxidation or methylation were attempted to elucidate the reaction conditions and mechanism. The heavier alkali and silver salts of the above‐mentioned heterocycle were isolated. The salts were characterized and investigated by means of NMR, vibrational spectroscopy, X‐ray diffraction and energetic properties.

Document Details

Document Type
Pub Defense Publication
Publication Date
Sep 18, 2017
Source ID
10.1002/prep.201700170

Entities

People

  • Burkhard Krumm
  • Thomas M. Klapötke
  • Tobias S. Hermann

Organizations

  • Ludwig-Maximilians-Universität München
  • Office of Naval Research

Tags

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry