Phase Contrast X‐Ray Imaging of the Collapse of an Engineered Void in Single‐Crystal HMX

Abstract

Imaging the collapse of a single void that creates a hot spot initiation site in an otherwise defect‐free explosive is challenging given the spatial and temporal scales involved in explosive systems. This work presents our attempt to examine a single hot spot mode (void collapse) in single‐crystal octahydro‐l,3,5,7‐tetranitro‐l,3,5,7‐tetrazocine (HMX) embedded in Sylgard. The hot spot heating mechanisms involved with pore collapse include adiabatic heating, jetting, and viscoplastic dissipation. Quantifying the dynamics of a pore collapse is a crucial step to understanding which mechanisms dominate during ignition events. Our experiments were conducted with a single‐stage, light‐gas gun at Argonne National Laboratory's Advanced Photon Source, applying the phase contrast imaging technique while collecting high‐speed video. The details of HMX single crystal production, defect (pore) engineering, and sample construction, along with experimental results are presented here. These results demonstrate that detailed collapse dynamics can be obtained from homogeneous, single‐crystal explosives with this approach. Qualitative comparisons are made with simulation data which show good agreement in the transition between a quasi‐symmetric pore collapse and an asymmetric collapse with jetting across the pore as measured with normalized pore area and pore circularity.

Document Details

Document Type
Pub Defense Publication
Publication Date
Aug 02, 2022
Source ID
10.1002/prep.202100297

Entities

People

  • Camilo A. Duarte
  • Christian J. Blum‐Sorensen
  • Jonathan D. Drake
  • Kamel Fezzaa
  • Marisol Koslowski
  • Nicholas E. Kerschen
  • Steven F Son
  • Weinong W. Chen

Organizations

  • Argonne National Laboratory
  • Lawrence Livermore National Laboratory
  • Purdue University

Tags

Fields of Study

  • Physics

Readers

  • Combustion Dynamics and Shock Wave Physics.
  • Materials Science (Mechanical Engineering).
  • Underwater engineering and Marine Technology.