Magnetic excitation and thermodynamics of BaFe2As2
Abstract
Magnetic excitation of the iron‐based superconductor parent compound BaFe2As2 at finite temperature are addressed with a first‐principles formulation of the Helmholtz energy, which can account for the finite temperature mixture of many magnetic configurations. We find that it is the spin exchange coupling in the interplane c direction that dictates the spin density wave ordering. We have also quantitatively predicted the pressure dependence of the spin density wave ordering temperature, the Schottky anomaly, and the temperature dependence of thermal populations of several low‐energy spin configurations, all in agreement with available experimental data. © 2010 Wiley Periodicals, Inc. Int J Quantum Chem, 2011
Document Details
- Document Type
- Pub Defense Publication
- Publication Date
- Oct 26, 2010
- Source ID
- 10.1002/qua.22865
Entities
People
- L. Q. Chen
- S. L. Shang
- Yaonan Wang
- Z. K. Liu
Organizations
- National Science Foundation
- Office of Naval Research
- Office of Science