Near‐Field Energy Transfer between a Luminescent 2D Material and Color Centers in Diamond

Abstract

Energy transfer between fluorescent probes lies at the heart of many applications ranging from bio‐sensing and bio‐imaging to enhanced photodetection and light harvesting. In this work, Förster resonance energy transfer (FRET) between shallow defects in diamond—nitrogen‐vacancy (NV) centers—and atomically thin, 2D materials—tungsten diselenide (WSe2)—is studied. By means of fluorescence lifetime imaging, the occurrence of FRET in the WSe2/NV system is demonstrated. Further, it is shown that in the coupled system, NV centers provide an additional excitation pathway for WSe2 photoluminescence. The results constitute the first step toward the realization of hybrid quantum systems involving single‐crystal diamond and 2D materials that may lead to new strategies for studying and controlling spin transfer phenomena and spin valley physics.

Document Details

Document Type
Pub Defense Publication
Publication Date
Nov 05, 2019
Source ID
10.1002/qute.201900088

Entities

People

  • Abdallah Slablab
  • Carlo Bradac
  • Chi Li
  • Elke Neu
  • Igor Aharonovich
  • Mariusz Radtke
  • Mehran Kianinia
  • Richard Nelz
  • Zai‐quan Xu

Organizations

  • Australian Research Council
  • Federal Ministry of Research, Technology and Space
  • Office of Naval Research Global
  • Saarland University
  • University of Technology Sydney

Tags

Fields of Study

  • Physics

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Nanoscale Plasmonic Nanotechnology
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Quantum Computing
  • Quantum Science - Quantum Dots