Synthesis and Characterization of Tetrahedral Zinc(II) Complexes with 3, 6,7‐Triamino‐7H‐[1, 2,4]triazolo[4, 3‐b][1, 2,4]triazole as Nitrogen‐Rich Ligand

Abstract

Triaminotriazolotriazole (TATOT) was used as a nitrogen‐rich ligand for the formation of the energetic ZnII complexes [ZnCl2(TATOT)2]·H2O (2), [Zn(H2O)(TATOT)3](NO3)2·2H2O (3), and [Zn(TATOT)4](ClO4)2·2H2O (4). The zinc species were prepared in a straightforward and inexpensive synthesis. The complexes 2–4 were structurally characterized using X‐ray diffraction. Additionally, the compounds were characterized using elemental analysis and infrared (IR) spectroscopy. Finally, the sensitivities toward thermal and mechanical stimuli were determined by differential thermal analysis (DTA) and BAM (Bundesanstalt für Materialforschung und ‐prüfung) methods.

Document Details

Document Type
Pub Defense Publication
Publication Date
Feb 29, 2016
Source ID
10.1002/zaac.201600006

Entities

People

  • Jörg Stierstorfer
  • Norbert Szimhardt
  • Philipp C. Schmid
  • Thomas M. Klapötke

Organizations

  • Office of Naval Research
  • United States Army Armament Research, Development and Engineering Center
  • United States Army Research Laboratory

Tags

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry
  • Positioning, Navigation, and Timing (PNT) Technology.