Per‐ and Polyfluoroalkyl Substances (PFAS) in Subsurface Environments: Occurrence, Fate, Transport, and Research Prospect

Abstract

Per‐ and polyfluoroalkyl substances (PFASs), also known as “forever chemicals,” are manmade chemicals that have been increasingly detected in various geological settings since the early 2000s. The soil and subsurface environments are the geological media commonly affected by PFAS. We conducted a comprehensive review of peer‐reviewed articles published from 2010 through 2022 concerning the fate and transport of PFAS in subsurface environments. This review is organized into different subsections, covering the basics of PFAS properties and how they affect the occurrence, fate, and transport of PFAS, the fundamental processes affecting subsurface transport and fate of PFAS, and mathematical models for describing and predicting PFAS transport behaviors. Mechanisms governing PFAS transport in the subsurface environment, including the sorption of PFAS at the air‐water interface, solid‐water interface, and nonaqueous phase liquids‐water interface, were explored in detail. Challenges and future research priorities are identified to better mitigate the global challenges of PFAS contamination.

Document Details

Document Type
Pub Defense Publication
Publication Date
Aug 18, 2022
Source ID
10.1029/2021rg000765

Entities

People

  • Chang Min Park
  • Chongyang Shen
  • Dengjun Wang
  • Feng Xiao
  • Jingjing Chen
  • Markus Flury
  • Yuanyuan Sun

Organizations

  • Auburn University
  • Kyungpook National University
  • Nanjing University
  • Nanjing University of Information Science and Technology
  • United States Department of Defense
  • University of Missouri
  • University of North Dakota
  • Virginia Tech
  • Washington State University

Tags

Fields of Study

  • Environmental science

Readers

  • Fire Suppression Systems Design.
  • Groundwater Contamination Remediation.
  • Technical Research and Report Writing.