Broadband 1-GHz mid-infrared frequency comb
Abstract
Mid-infrared (MIR) spectrometers are invaluable tools for molecular fingerprinting and hyper-spectral imaging. Among the available spectroscopic approaches, GHz MIR dual-comb absorption spectrometers have the potential to simultaneously combine the high-speed, high spectral resolution, and broad optical bandwidth needed to accurately study complex, transient events in chemistry, combustion, and microscopy. However, such a spectrometer has not yet been demonstrated due to the lack of GHz MIR frequency combs with broad and full spectral coverage. Here, we introduce the first broadband MIR frequency comb laser platform at 1 GHz repetition rate that achieves spectral coverage from 3 to 13 µm. This frequency comb is based on a commercially available 1.56 µm mode-locked laser, robust all-fiber Er amplifiers and intra-pulse difference frequency generation (IP-DFG) of few-cycle pulses in χ(2) nonlinear crystals. When used in a dual comb spectroscopy (DCS) configuration, this source will simultaneously enable measurements with μs time resolution, 1 GHz (0.03 cm−1) spectral point spacing and a full bandwidth of >5 THz (>166 cm−1) anywhere within the MIR atmospheric windows. This represents a unique spectroscopic resource for characterizing fast and non-repetitive events that are currently inaccessible with other sources.
Document Details
- Document Type
- Pub Defense Publication
- Publication Date
- Sep 07, 2022
- Source ID
- 10.1038/s41377-022-00947-w
Entities
People
- Alexander Lind
- Daniel Lesko
- Greg Rieker
- Nazanin Hoghooghi
- Peter Chang
- Scott A. Diddams
- Sida Xing
Organizations
- Air Force Office of Scientific Research
- National Institute of Standards and Technology
- National Science Foundation
- United States Department of Defense