Emerging photoluminescence from the dark-exciton phonon replica in monolayer WSe2

Abstract

Tungsten-based monolayer transition metal dichalcogenides host a long-lived “dark” exciton, an electron-hole pair in a spin-triplet configuration. The long lifetime and unique spin properties of the dark exciton provide exciting opportunities to explore light-matter interactions beyond electric dipole transitions. Here we demonstrate that the coupling of the dark exciton and an optically silent chiral phonon enables the intrinsic photoluminescence of the dark-exciton replica in monolayer WSe2. Gate and magnetic-field dependent PL measurements unveil a circularly-polarized replica peak located below the dark exciton by 21.6 meV, equal to E″ phonon energy from Se vibrations. First-principles calculations show that the exciton-phonon interaction selectively couples the spin-forbidden dark exciton to the intravalley spin-allowed bright exciton, permitting the simultaneous emission of a chiral phonon and a circularly-polarized photon. Our discovery and understanding of the phonon replica reveals a chirality dictated emission channel of the phonons and photons, unveiling a new route of manipulating valley-spin.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jun 06, 2019
Source ID
10.1038/s41467-019-10477-6

Entities

People

  • Chenhao Jin
  • Dmitry Smirnov
  • Kenji Watanabe
  • Mark Blei
  • Sefaattin Tongay
  • Shiyuan Gao
  • Su-Fei Shi
  • Takashi Taniguchi
  • Tianhui Ren
  • Tianmeng Wang
  • Ting Cao
  • Yang Li
  • Yuze Meng
  • Zhen Lian
  • Zhengguang Lu
  • Zhipeng Li

Organizations

  • Air Force Office of Scientific Research

Tags

Fields of Study

  • Physics

Readers

  • Quantum Chemistry
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene
  • Quantum Science - Quantum Dots