Competing correlated states and abundant orbital magnetism in twisted monolayer-bilayer graphene

Abstract

Flat band moiré superlattices have recently emerged as unique platforms for investigating the interplay between strong electronic correlations, nontrivial band topology, and multiple isospin ‘flavor’ symmetries. Twisted monolayer-bilayer graphene (tMBG) is an especially rich system owing to its low crystal symmetry and the tunability of its bandwidth and topology with an external electric field. Here, we find that orbital magnetism is abundant within the correlated phase diagram of tMBG, giving rise to the anomalous Hall effect in correlated metallic states nearby most odd integer fillings of the flat conduction band, as well as correlated Chern insulator states stabilized in an external magnetic field. The behavior of the states at zero field appears to be inconsistent with simple spin and valley polarization for the specific range of twist angles we investigate, and instead may plausibly result from an intervalley coherent (IVC) state with an order parameter that breaks time reversal symmetry. The application of a magnetic field further tunes the competition between correlated states, in some cases driving first-order topological phase transitions. Our results underscore the rich interplay between closely competing correlated ground states in tMBG, with possible implications for probing exotic IVC ordering.

Document Details

Document Type
Pub Defense Publication
Publication Date
Aug 05, 2021
Source ID
10.1038/s41467-021-25044-1

Entities

People

  • Kenji Watanabe
  • Matthew Yankowitz
  • Minhao He
  • Takashi Taniguchi
  • Xiaodong Xu
  • Ya-hui Zhang
  • Yuhao Li
  • Zaiyao Fei

Organizations

  • Army Research Office
  • Core Research for Evolutional Science and Technology
  • Division of Materials Research
  • Japan Society for the Promotion of Science
  • Ministry of Education, Culture, Sports, Science and Technology
  • National Science Foundation

Tags

Fields of Study

  • Physics

Readers

  • Educational Psychology
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene
  • Space