Architecture for microcomb-based GHz-mid-infrared dual-comb spectroscopy

Abstract

Dual-comb spectroscopy (DCS) offers high sensitivity and wide spectral coverage without the need for bulky spectrometers or mechanical moving parts. And DCS in the mid-infrared (mid-IR) is of keen interest because of inherently strong molecular spectroscopic signatures in these bands. We report GHz-resolution mid-IR DCS of methane and ethane that is derived from counter-propagating (CP) soliton microcombs in combination with interleaved difference frequency generation. Because all four combs required to generate the two mid-IR combs rely upon stability derived from a single high-Q microcavity, the system architecture is both simplified and does not require external frequency locking. Methane and ethane spectra are measured over intervals as short as 0.5 ms, a time scale that can be further reduced using a different CP soliton arrangement. Also, tuning of spectral resolution on demand is demonstrated. Although at an early phase of development, the results are a step towards mid-IR gas sensors with chip-based architectures for chemical threat detection, breath analysis, combustion studies, and outdoor observation of trace gases.

Document Details

Document Type
Pub Defense Publication
Publication Date
Nov 12, 2021
Source ID
10.1038/s41467-021-26958-6

Entities

People

  • Chengying Bao
  • Heming Wang
  • Kerry Vahala
  • Lue Wu
  • Myoung-Gyun Suh
  • Qiang Lin
  • Zhiquan Yuan

Organizations

  • Air Force Research Laboratory Information Directorate
  • Defense Threat Reduction Agency

Tags

Readers

  • Analytical Chemistry
  • Optical Physics and Photonics.
  • Radio communications and signal processing.