Wide field imaging of van der Waals ferromagnet Fe3GeTe2 by spin defects in hexagonal boron nitride

Abstract

Emergent color centers with accessible spins hosted by van der Waals materials have attracted substantial interest in recent years due to their significant potential for implementing transformative quantum sensing technologies. Hexagonal boron nitride (hBN) is naturally relevant in this context due to its remarkable ease of integration into devices consisting of low-dimensional materials. Taking advantage of boron vacancy spin defects in hBN, we report nanoscale quantum imaging of low-dimensional ferromagnetism sustained in Fe3GeTe2/hBN van der Waals heterostructures. Exploiting spin relaxometry methods, we have further observed spatially varying magnetic fluctuations in the exfoliated Fe3GeTe2 flake, whose magnitude reaches a peak value around the Curie temperature. Our results demonstrate the capability of spin defects in hBN of investigating local magnetic properties of layered materials in an accessible and precise way, which can be extended readily to a broad range of miniaturized van der Waals heterostructure systems.

Document Details

Document Type
Pub Defense Publication
Publication Date
Sep 13, 2022
Source ID
10.1038/s41467-022-33016-2

Entities

People

  • Chunhui Du
  • Di Chen
  • Dziga Djugba
  • Hailong Wang
  • Hanyi Lu
  • Jing Shi
  • Jingcheng Zhou
  • Mengqi Huang
  • Mohammed Alghamdi
  • Nathan J. McLaughlin
  • Senlei Li

Organizations

  • Air Force Office of Scientific Research
  • National Science Foundation

Tags

Fields of Study

  • Physics

Readers

  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Quantum Computing
  • Quantum Science - Quantum Dots