Oxygen-induced changes to selectivity-determining steps in electrocatalytic CO2 reduction

Abstract

The state of the electrocatalyst surface—including the oxidation state of the catalyst and the presence of spectator species—is investigated on Cu surfaces with density functional theory in order to understand predicted ramifications on the selectivity of CO2 reduction between CH4 and CH3OH.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jan 01, 2015
Source ID
10.1039/c4cp03783a

Entities

People

  • Andrew A Peterson
  • Yin-jia Zhang

Organizations

  • Brown University
  • Office of Naval Research
  • United States Army
  • Yusuf Hamied Department of Chemistry

Tags

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Game Theory.
  • Mathematics or Statistics

Technology Areas

  • Microelectronics