σ-Aromaticity in polyhydride complexes of Ru, Ir, Os, and Pt

Abstract

Transition-metal hydrides are essential for catalysis, organic synthesis, and hydrogen storage. In this work we study IrH5(PPh3)2, (RuH5(PiPr3)2)−, (OsH5(PiPr3)2)−, and OsH4(PPhMe2)3 polyhydride complexes, where the metal is five-fold coordinated in-plane. The unusual coordination of these compounds can be explained by σ-aromaticity.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jan 01, 2016
Source ID
10.1039/c5cp04330a

Entities

People

  • Anastassia N. Alexandrova
  • Elisa Jimenez-Izal

Organizations

  • Air Force Office of Scientific Research
  • California NanoSystems Institute
  • National Science Foundation Directorate for Biological Sciences
  • United States Army
  • University of California
  • Yusuf Hamied Department of Chemistry

Tags

Fields of Study

  • Chemistry

Readers

  • Electrical Engineering
  • Electrochemical Surface Science
  • Organic Chemistry