Two-step model for ultrafast interfacial electron transfer: limitations of Fermi’s golden rule revealed by quantum dynamics simulations
Abstract
A two-step model of interfacial electron transfer is proposed along with a practical approach to screening dye-sensitizers based on a calculation of the percentage of electron density on the linker group and the number of available semiconductor acceptor states.
Document Details
- Document Type
- Pub Defense Publication
- Publication Date
- Jan 01, 2017
- Source ID
- 10.1039/c7sc01169e
Entities
People
- Chang Liu
- Elena Jakubikova
Organizations
- Army Research Office
- North Carolina State University
- United States Army
- Yusuf Hamied Department of Chemistry