A quantum molecular movie: polyad predissociation dynamics in the VUV excited 3pσ2Σu state of NO2

Abstract

We present time-resolved photoelectron spectroscopy studies of an electronically excited triatomic molecule wherein the vibrational dynamics must be treated quantum mechanically and the simple picture of population flow between coupled normal modes fails.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jan 01, 2021
Source ID
10.1039/d0fd00128g

Entities

People

  • Albert Stolow
  • Andrey E. Boguslavskiy
  • Edward R. Grant
  • Iain Wilkinson
  • Kevin Veyrinas
  • Michael S Schuurman
  • Ruaridh Forbes
  • Rune Lausten
  • Varun Makhija

Organizations

  • Air Force Office of Scientific Research
  • Engineering and Physical Sciences Research Council
  • Helmholtz-Zentrum Berlin
  • National Research Council Canada
  • Natural Sciences and Engineering Research Council
  • SLAC National Accelerator Laboratory
  • United States Army
  • University of British Columbia
  • University of Mary Washington
  • University of Ottawa
  • Yusuf Hamied Department of Chemistry

Tags

Fields of Study

  • Physics

Readers

  • Atmospheric Science / Meteorology, specifically Wind Wave Turbulence.
  • Molecular Photonics/Laser Physics

Technology Areas

  • Microelectronics
  • Quantum Computing