Surface segregation effects of erbium in GaAs growth and their implications for optical devices containing ErAs nanostructures

Abstract

We report on the integration of semimetallic ErAs nanoparticles with high optical quality GaAs-based semiconductors, grown by molecular beam epitaxy. Secondary ion mass spectrometry and photoluminescence measurements provide evidence of surface segregation and incorporation of erbium into layers grown with the erbium cell hot, despite the closed erbium source shutter. We establish the existence of a critical areal density of the surface erbium layer, below which the formation of ErAs precipitates is suppressed. Based upon these findings, we demonstrate a method for overgrowing ErAs nanoparticles with III-V layers of high optical quality, using subsurface ErAs nanoparticles as a sink to deplete the surface erbium concentration. This approach provides a path toward realizing optical devices based on plasmonic effects in an epitaxially-compatible semimetal/semiconductor system.

Document Details

Document Type
Pub Defense Publication
Publication Date
Mar 21, 2011
Source ID
10.1063/1.3565168

Entities

People

  • Adam M. Crook
  • Hari P. Nair
  • Seth R. Bank

Organizations

  • Air Force Office of Scientific Research
  • Army Research Office
  • University of Texas at Austin

Tags

Fields of Study

  • Materials science

Readers

  • Optical Physics and Photonics.
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Biotechnology
  • Microelectronics