Photothermal-reaction-assisted two-photon lithography of silver nanocrystals capped with thermally cleavable ligands

Abstract

We report an alternative approach to produce micropatterns of metallic nanoparticles using photothermal-reaction-assisted two-photon direct laser writing. The patterns are achieved using a facile surface treatment of silver nanoparticles (Ag NPs) functionalized with thermally cleavable ligands; N-(tert-butoxycarbonyl)-L-cysteine methyl ester. The ligand cleavage initiated by pulsed laser-induced thermal reaction results in a significant change in dispersiblility of the nanocrystals, thereby enabling a solvent-selective development process after photopatterning. We demonstrated that Ag NP patterns with submicron linewidths can be achieved using near infrared pulsed laser illumination.

Document Details

Document Type
Pub Defense Publication
Publication Date
Mar 28, 2011
Source ID
10.1063/1.3565245

Entities

People

  • Alexander Baev
  • Hong Sub Jee
  • Mark T. Swihart
  • Paras Nath Prasad
  • Won Jin Kim
  • Xavier Vidal

Organizations

  • Air Force Office of Scientific Research
  • University at Buffalo

Tags

Readers

  • Nanocomposite Materials Science
  • Optical Physics and Photonics.
  • Polymer Science and Engineering.

Technology Areas

  • Biotechnology
  • Directed Energy