Site-selective spectroscopy and crystal-field analysis for Nd3+ in strontium fluorovanadate

Abstract

Site-selective spectroscopy reveals that Nd3+ ions occupy more than 40 different crystal-field environments in Sr5(VO4)3F. Preferential energy transfer to the site responsible for 1 μm lasing occurs but becomes less complete with increasing temperature. The 4I and 4F3/2 Stark levels of the lasing site have been determined and an analysis of the crystal field performed. From the crystal-field fitting parameters Bkq, a calculated energy-level spectrum is determined up to 17 500 cm−1 with a rms deviation from the available experimental levels of 6 cm−1.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jan 01, 1995
Source ID
10.1063/1.359387

Entities

People

  • B. H. T. Chai
  • C. A. Morrison
  • H. Weidner
  • P. L. Summers
  • Robert E. Peale

Organizations

  • United States Army Research Laboratory
  • University of Central Florida

Tags

Fields of Study

  • Physics

Readers

  • Educational Psychology
  • Materials Science and Engineering.
  • Molecular Photonics/Laser Physics