Multi-reference Fock space coupled-cluster method in the intermediate Hamiltonian formulation for potential energy surfaces

Abstract

The effective and intermediate Hamiltonian multi-reference coupled-cluster (CC) method with singles and doubles for the doubly ionized (0,2) sector of Fock space (FS) is formulated and implemented. The intermediate Hamiltonian realization of the (0,2) FS problem provides a robust computational scheme for solving the FS-CC equations free from the intruder state problem. By introducing an efficient factorization strategy, we obtain a very efficient tool that can be used for computing double ionization potentials but more significantly to describe multi-reference problems in CC theory, illustrated by twisted ethylene and the potential energy curve for F2. The latter separates smoothly to two F atoms, while the former avoids the cusp behavior at the 90° dihedral. We also explore the double ionization potentials for several small molecules, H2O, CO, C2H2, and C2H4.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jul 28, 2011
Source ID
10.1063/1.3615500

Entities

People

  • Monika Musiał
  • Rodney J. Bartlett

Organizations

  • Air Force Office of Scientific Research
  • University of Florida
  • University of Silesia in Katowice

Tags

Readers

  • Adaptive Control and Estimation with Uncertainty in Dynamic Systems.
  • Organic Chemistry
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Space