Direct measurements of collisionally broadened Raman linewidths of CO2 S-branch transitions

Abstract

We report direct measurements of S-branch Raman-coherence lifetimes of CO2 resulting from CO2–CO2 and CO2–N2 collisions by employing time-resolved picosecond coherent anti-Stokes Raman scattering spectroscopy. The S-branch (ΔJ = +2) transitions of CO2 with rotational quantum number J = 0–52 were simultaneously excited using a broadband (∼5 nm) laser pulse with a full-width-at-half-maximum duration of ∼115 ps. The coherence lifetimes of CO2 for a pressure range of 0.05–1 atm were measured directly by probing the rotational coherence with a nearly transform-limited, 90-ps-long laser pulse. These directly measured Raman-coherence lifetimes, when converted to collisional linewidth broadening coefficients, differ from the previously reported broadening coefficients extracted from frequency-domain rotational Raman and infrared-absorption spectra and from theoretical calculations by 7%–25%.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jan 10, 2013
Source ID
10.1063/1.4774093

Entities

People

  • Hans U. Stauffer
  • James. R. Gord
  • Joseph R. Gord
  • Naibo Jiang
  • Paul S. Hsu
  • Sukesh Roy
  • Waruna D. Kulatilaka

Organizations

  • Air Force Office of Scientific Research
  • Air Force Research Laboratory
  • Purdue University

Tags

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Molecular Photonics/Laser Physics
  • Optical Physics and Photonics.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Quantum Computing