Communication: One-photon phase control of cis-trans isomerization in retinal

Abstract

We computationally demonstrate the one-photon phase control of retinal isomerization under conditions of low laser intensity. The calculations, utilizing the multiconfigurational time dependent Hartree method, include coupling between the two modes that are active in isomerization and the background molecular vibrational environment. Noting previously unsuccessful computations highlights the significance of this result.

Document Details

Document Type
Pub Defense Publication
Publication Date
Feb 21, 2013
Source ID
10.1063/1.4792834

Entities

People

  • Carlos A. Arango
  • Paul Brumer

Organizations

  • Air Force Office of Scientific Research
  • Universidad Icesi
  • University of Toronto

Tags

Fields of Study

  • Physics

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Quantum Chemistry
  • Systems Analysis and Design

Technology Areas

  • Directed Energy