Two color pumping of the Rb D2 line laser (780 nm) through the photoassociation of Rb-Ar or Rb-Xe thermal pairs: Realization of a quantum efficiency above one

Abstract

A two color process for optical pumping of the Rb D2 line laser (λ = 780 nm) in Rb vapor-rare gas mixtures is demonstrated to yield an overall quantum efficiency > 1. Combining photoexcitation of the Rb D2 line blue satellite in Rb-Xe or Rb-Ar mixtures with free ← free optical pumping of the A2Π12←X2Σ12+ transition at large internuclear separation (R > 5 Å) also increases the laser efficiency and pump absorption coefficient, relative to the single color, B ← X pumped system, by a factor of 1.7 and more than an order of magnitude, respectively. Simultaneous photopumping of Rb-Xe thermal collision pairs at 760 nm (D2 satellite) and 794.3 nm results in a 780 nm (D2 line) laser with a quantum efficiency of 1.008 which corresponds to the removal of ∼102 cm–1 (12.6 meV) of thermal energy per emitted photon.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jul 27, 2015
Source ID
10.1063/1.4927536

Entities

People

  • A E Mironov
  • James Gary Eden
  • William Goldshlag

Organizations

  • Air Force Office of Scientific Research
  • University of Illinois Urbana–Champaign

Tags

Fields of Study

  • Engineering
  • Physics

Readers

  • Molecular Photonics/Laser Physics
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Quantum Computing
  • Space
  • Space - Hall-Effect Thruster