Approximating electronically excited states with equation-of-motion linear coupled-cluster theory

Abstract

A new perturbative approach to canonical equation-of-motion coupled-cluster theory is presented using coupled-cluster perturbation theory. A second-order Møller-Plesset partitioning of the Hamiltonian is used to obtain the well known equation-of-motion many-body perturbation theory equations and two new equation-of-motion methods based on the linear coupled-cluster doubles and linear coupled-cluster singles and doubles wavefunctions. These new methods are benchmarked against very accurate theoretical and experimental spectra from 25 small organic molecules. It is found that the proposed methods have excellent agreement with canonical equation-of-motion coupled-cluster singles and doubles state for state orderings and relative excited state energies as well as acceptable quantitative agreement for absolute excitation energies compared with the best estimate theory and experimental spectra.

Document Details

Document Type
Pub Defense Publication
Publication Date
Oct 23, 2015
Source ID
10.1063/1.4934232

Entities

People

  • Ajith Perera
  • Jason N. Byrd
  • Rodney J. Bartlett
  • Varun Rishi

Organizations

  • Air Force Office of Scientific Research
  • Army Research Office
  • Max Planck Society
  • University of Florida

Tags

Fields of Study

  • Physics

Readers

  • Computational Modeling and Simulation
  • Graph Algorithms and Convex Optimization.
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Microelectronics