Communication: Enhanced dissociative chemisorption of CO2 via vibrational excitation

Abstract

A fully coupled global nine-dimensional potential energy surface for the dissociative chemisorption of CO2 on Ni(100) is constructed from ∼18 000 density functional points. It reveals a complex reaction pathway dominated by two near iso-energetic transition states. The dissociation probabilities obtained by quasi-classical trajectories on the potential energy surface reproduced experimental trends, and indicate that vibrational excitations of CO2 significantly promote the dissociation. Using the sudden vector projection model, the behavior of the reactivity is rationalized by couplings with the reaction coordinate at each transition state. These results offer plausible rationalization for the observed enhancement of CO2 dissociation in non-thermal plasmas by metal surfaces.

Document Details

Document Type
Pub Defense Publication
Publication Date
Mar 01, 2016
Source ID
10.1063/1.4943002

Entities

People

  • Bin Jiang
  • Hua Guo

Organizations

  • Air Force Office of Scientific Research
  • National Natural Science Foundation of China
  • National Science Foundation
  • University of New Mexico
  • University of Science and Technology of China

Tags

Fields of Study

  • Physics

Readers

  • Computer Vision.
  • Molecular Photonics/Laser Physics
  • Quantum Chemistry