Blind test of density-functional-based methods on intermolecular interaction energies

Abstract

In the past decade, a number of approaches have been developed to fix the failure of (semi)local density-functional theory (DFT) in describing intermolecular interactions. The performance of several such approaches with respect to highly accurate benchmarks is compared here on a set of separation-dependent interaction energies for ten dimers. Since the benchmarks were unknown before the DFT-based results were collected, this comparison constitutes a blind test of these methods.

Document Details

Document Type
Pub Defense Publication
Publication Date
Sep 23, 2016
Source ID
10.1063/1.4961095

Entities

People

  • Cui Zhang
  • Decarlos E. Taylor
  • Donald Truhlar
  • François Gygi
  • Giulia Galli
  • Gustavo E. Scuseria
  • Ireneusz Bulik
  • Jong Won Song
  • Julien Toulouse
  • János Ángyán
  • Kar Rahul
  • Kimihiko Hirao
  • Krzysztof Szalewicz
  • O Anatole von Lilienfeld
  • Rafał Podeszwa
  • Roberto Peverati
  • Thomas M. Henderson

Organizations

  • Army Research Office
  • Florida Institute of Technology
  • National Science Foundation
  • Pierre and Marie Curie University
  • RIKEN Center for Computational Science
  • Rice University
  • United States Army Research Laboratory
  • United States Department of Energy
  • University of Basel
  • University of California
  • University of California, Davis
  • University of Chicago
  • University of Delaware
  • University of Lorraine
  • University of Minnesota
  • University of Silesia in Katowice
  • Vrije Universiteit Brussel

Tags

Readers

  • Computer Vision.
  • Quantum Chemistry
  • Regression Analysis.