Adsorption-controlled growth of La-doped BaSnO3 by molecular-beam epitaxy

Abstract

Epitaxial La-doped BaSnO3 films were grown in an adsorption-controlled regime by molecular-beam epitaxy, where the excess volatile SnOx desorbs from the film surface. A film grown on a (001) DyScO3 substrate exhibited a mobility of 183 cm2 V−1 s−1 at room temperature and 400 cm2 V−1 s−1 at 10 K despite the high concentration (1.2 × 1011 cm−2) of threading dislocations present. In comparison to other reports, we observe a much lower concentration of (BaO)2 Ruddlesden-Popper crystallographic shear faults. This suggests that in addition to threading dislocations, other defects—possibly (BaO)2 crystallographic shear defects or point defects—significantly reduce the electron mobility.

Document Details

Document Type
Pub Defense Publication
Publication Date
Nov 01, 2017
Source ID
10.1063/1.5001839

Entities

People

  • Amit Verma
  • Ariel Seidner H.
  • Bi-Cheng Zhou
  • Darrell G. Schlom
  • David A. Muller
  • Debdeep Jena
  • Edward B. Lochocki
  • Hanjong Paik
  • Jisung Park
  • Kyle. M. Shen
  • Mario Brützam
  • Masaki Uchida
  • Nicholas Tanen
  • Reinhard Uecker
  • Shunli Shang
  • Zhen Chen
  • Zi-Kui Liu

Organizations

  • Air Force Office of Scientific Research
  • Cornell University
  • Indian Institute of Technology Kanpur
  • Leibniz Institute for Crystal Growth
  • National Science Foundation
  • Pennsylvania State University
  • University of Tokyo

Tags

Fields of Study

  • Materials science

Readers

  • Canadian European Scientific Immigration and Epilepsy Clearance Studies
  • Materials Science and Engineering.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene