Growth and electronic properties of nanolines on TiO2-terminated SrTiO3(001) surfaces

Abstract

Surfaces of homoepitaxially grown TiO2-terminated SrTiO3(001) were studied in situ with scanning tunneling microscopy and spectroscopy. By controlling the Ti/Sr ratio, two-dimensional domains of highly ordered linear nanostructures, so-called “nanolines,” are found to form on the surface. To further study how the surface structure affects the band structure, spectroscopic studies of these surfaces were performed. Our results reveal significantly more band bending for surfaces with the nanolines, indicative of an acceptor state associated with these features. Additionally, an in-gap state is observed on nanoline surfaces grown under high oxygen deficient conditions. This state appears to be the same as that observed previously, arising from the (++/+) transition level of surface oxygen vacancies.

Document Details

Document Type
Pub Defense Publication
Publication Date
Sep 27, 2017
Source ID
10.1063/1.5004982

Entities

People

  • Marek Skowronski
  • Randall M. Feenstra
  • W. Sitaputra
  • Wei Yan

Organizations

  • Air Force Office of Scientific Research
  • Carnegie Mellon University

Tags

Fields of Study

  • Physics

Readers

  • Nanoscale Plasmonic Nanotechnology
  • Semiconductor Device Technology
  • Theoretical Analysis.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene