High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

Abstract

Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606–611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.

Document Details

Document Type
Pub Defense Publication
Publication Date
May 01, 2018
Source ID
10.1063/1.5017908

Entities

People

  • A. J. Mackinnon
  • A. K. Schuster
  • A. Pak
  • A. Pelka
  • A. Ravasio
  • A. Zettl
  • Alejandro Laso Garcia
  • Alison Saunders
  • D. O. Gericke
  • Dominik Kraus
  • E. Cunningham
  • E. Galtier
  • E. Granados
  • E. J. Gamboa
  • Emma Elizabeth Mcbride
  • H. J. Lee
  • I. Nam
  • I. Prencipe
  • J. Vorberger
  • K. Rohatsch
  • L. B. Fletcher
  • M. Rödel
  • M. Schölmerich
  • M. Schörner
  • Michael Macdonald
  • Nicholas Hartley
  • P. Neumayer
  • Peihao Sun
  • Philip Heimann
  • R. W. Falcone
  • Ronald Redmer
  • S. Frydrych
  • S. J. Turner
  • Shaughnessy Brennan Brown
  • Siegfried Glenzer
  • T. Döppner
  • Thomas E. Cowan
  • Tim B Van Driel

Organizations

  • Air Force Office of Scientific Research
  • European XFEL
  • Federal Ministry of Research, Technology and Space
  • GSI Helmholtz Centre for Heavy Ion Research
  • German Research Foundation
  • Helmholtz Association of German Research Centres
  • Helmholtz-Zentrum Dresden-Rossendorf
  • Japan Society for the Promotion of Science
  • Lawrence Berkeley National Laboratory
  • Lawrence Livermore National Laboratory
  • Osaka University
  • SLAC National Accelerator Laboratory
  • Technical University of Darmstadt
  • United States Department of Energy
  • University of Michigan
  • University of Rostock
  • University of Warwick

Tags

Fields of Study

  • Physics

Readers

  • Mechanical Engineering/Mechanics of Materials.
  • Nanoscale Plasmonic Nanotechnology
  • Ocean-Atmosphere Mesoscale Modeling, Data Assimilation, and Flux Boundary Layers

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers