Effective charges and zeta potentials of oil in water microemulsions in the presence of Hofmeister salts

Abstract

We present a theory which allows us to calculate the effective charge and zeta potential of oil droplets in microemulsions containing Hofmeister salts. A modified Poisson-Boltzmann equation is used to account for the surface and ion polarizations and hydrophobic and dispersion interactions. The ions are classified as kosmotropes and chaotropes according to their Jones-Dole viscosity B coefficient. Kosmotropes stay hydrated and do not enter into the oil phase, while chaotropes can adsorb to the oil-water interface. The effective interaction potentials between ions and oil-water interface are parametrized so as to accurately account for the excess interfacial tension.

Document Details

Document Type
Pub Defense Publication
Publication Date
Mar 16, 2018
Source ID
10.1063/1.5019704

Entities

People

  • Alexandre P dos Santos
  • Yan Levin

Organizations

  • Alexander von Humboldt Foundation
  • Coordenação de Aperfeicoamento de Pessoal de Nível Superior
  • Federal University of Rio Grande do Sul
  • Freie Universität Berlin
  • National Council for Scientific and Technological Development
  • United States Air Force

Tags

Fields of Study

  • Physics

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Marine Ecotoxicology
  • Plasma Physics.