Printed, 1 V electrolyte-gated transistors based on poly(3-hexylthiophene) operating at >10 kHz on plastic

Abstract

Electrolyte-gated transistors (EGTs) based on poly(3-hexylthiophene) (P3HT) offer low voltage operation, high transconductance, good operational stability, and low contact resistance. These characteristics derive from the massive electrochemical or double layer capacitance (∼10–100 μF/cm2) of the electrolyte layer that serves as the gate dielectric. However, electric double layer (EDL) formation at the source/electrolyte and drain/electrolyte interfaces results in significant parasitic capacitance in EGTs which degrades dynamic switching performance. Parasitic capacitance in EGTs is reduced by covering the top surfaces of the source/drain electrodes with a low-ĸ dielectric (∼0.6 nF/cm2). The low-ĸ dielectric blocks EDL formation on the electrode surfaces that are in direct contact with the gate electrolyte, reducing the parasitic capacitance by a factor of 104 and providing a route to printed P3HT EGTs on plastic operating at switching frequencies exceeding 10 kHz with 1 V supply voltages.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jul 30, 2018
Source ID
10.1063/1.5025475

Entities

People

  • C. Daniel Frisbie
  • Donghoon Song
  • Fazel Zare Bidoky
  • Woo Jin Hyun

Organizations

  • National Science Foundation
  • Office of Naval Research
  • University of Minnesota

Tags

Fields of Study

  • Materials science

Readers

  • Battery Technology and Engineering
  • Microwave Engineering.
  • Semiconductor Device Technology