Non-equilibrium stationary coherences in photosynthetic energy transfer under weak-field incoherent illumination

Abstract

We present a theoretical study of the quantum dynamics of energy transfer in a model photosynthetic dimer excited by incoherent light and show that the interplay between incoherent pumping and phonon-induced relaxation, dephasing, and trapping leads to the emergence of non-equilibrium stationary states characterized by substantial stationary coherences in the energy basis. We obtain analytic expressions for these coherences in the limits of rapid dephasing of electronic excitations and of small excitonic coupling between the chromophores. The stationary coherences are maximized in the regime where the excitonic coupling is small compared to the trapping rate. We further show that the non-equilibrium coherences anti-correlate with the energy transfer efficiency in the regime of localized coupling to the reaction center and that no correlation exists under delocalized (Förster) trapping conditions.

Document Details

Document Type
Pub Defense Publication
Publication Date
Mar 27, 2018
Source ID
10.1063/1.5028121

Entities

People

  • Paul Brumer
  • Timur V. Tscherbul

Organizations

  • Air Force Office of Scientific Research
  • University of Nevada, Reno
  • University of Toronto

Tags

Fields of Study

  • Physics

Readers

  • Calculus or Mathematical Analysis
  • Chemistry (specifically Chemical Fluorescence)
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Microelectronics
  • Quantum Computing
  • Quantum Science - Quantum Dots