Atomic layer deposition of epitaxial ferroelectric barium titanate on Si(001) for electronic and photonic applications

Abstract

Epitaxial barium titanate (BTO) thin films are grown on strontium titanate-buffered Si(001) using atomic layer deposition (ALD) at 225 °C. X-ray diffraction confirms compressive strain in BTO films after the low temperature growth for films as thick as 66 nm, with the BTO c-axis oriented in the out-of-plane direction. Postdeposition annealing above 650 °C leads to an in-plane c-axis orientation. Piezoresponse force microscopy was used to verify the ferroelectric switching behavior of ALD-grown films. Electrical and electro-optic measurements confirm BTO film ferroelectric behavior in out-of-plane and in-plane directions, respectively, at the micrometer scale.

Document Details

Document Type
Pub Defense Publication
Publication Date
Aug 08, 2019
Source ID
10.1063/1.5087571

Entities

People

  • Agham Posadas
  • Alexander A Demkov
  • Edward L. Lin
  • J. Elliott Ortmann
  • Jean Fompeyrine
  • John G Ekerdt
  • Keji Lai
  • Lu Zheng
  • Stefan Abel

Organizations

  • Air Force Office of Scientific Research
  • European Commission
  • International Business Machines Corporation (Armonk, NY)
  • National Science Foundation
  • National Science Foundation Directorate for Mathematical & Physical Sciences
  • University of Texas at Austin

Tags

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Thin Film Deposition Science.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene