Surface-induced thickness limit of conducting La-doped SrTiO3 thin films

Abstract

We report on a surface-induced, insulating, electrically dead layer in ultrathin conducting La-doped SrTiO3 thin films. Systematic studies on electrical properties as a function of film thickness and La-doping levels reveal that the insulating layer has a constant thickness and traps a constant amount of electron density regardless of La-doping levels. Growing an additional capping layer on top of the La-doped SrTiO3 surface counteracts the reduced conductivity, indicating a strong relationship between the insulating layer and the surface structure. Our results emphasize the importance of surface state studies for functional oxides in the thin film limit and provide a guiding principle for the fabrication of La-doped SrTiO3-based oxide nanoscale devices.

Document Details

Document Type
Pub Defense Publication
Publication Date
Oct 14, 2019
Source ID
10.1063/1.5111771

Entities

People

  • Charles Ahn
  • Claudia Lau
  • Frederick J. Walker
  • Sangjae Lee
  • Yeong Jae Shin

Organizations

  • Air Force Office of Scientific Research
  • Argonne National Laboratory
  • Office of Naval Research
  • Yale University

Tags

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Mathematics or Statistics
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Biotechnology
  • Microelectronics
  • Microelectronics - Graphene