Optical properties of cubic boron arsenide

Abstract

The ultrahigh thermal conductivity of cubic boron arsenide (BAs) makes it a promising material for next-generation electronics and optoelectronics. Here, we report measured optical properties of BAs crystals, including the complex dielectric function, refractive index, and absorption coefficient in the ultraviolet, visible, and near-infrared wavelength range. The data were collected at room temperature using spectroscopic ellipsometry and transmission and reflection spectroscopy. We further calculated the optical response using density functional theory and many-body perturbation theory, considering quasiparticle and excitonic corrections. The computed values for the direct and indirect bandgaps (4.25 eV and 2.07 eV) agree well with the measured results (4.12 eV and 2.02 eV). Our findings pave the way for using BAs in future electronic and optoelectronic applications that take advantage of its demonstrated ultrahigh thermal conductivity and predicted high ambipolar carrier mobility.

Document Details

Document Type
Pub Defense Publication
Publication Date
Apr 06, 2020
Source ID
10.1063/5.0004666

Entities

People

  • Bai Song
  • Emmanouil Kioupakis
  • Fei Tian
  • Gang Chen
  • Geethal Amila Gamage Udalamatta Gamage
  • Ke Chen
  • Kelsey Mengle
  • Kyle Bushick
  • Zhifeng Ren

Organizations

  • Massachusetts Institute of Technology
  • National Science Foundation
  • Office of Naval Research
  • Peking University
  • United States Department of Energy
  • University of Houston
  • University of Michigan

Tags

Fields of Study

  • Materials science
  • Physics

Readers

  • Materials Science and Engineering.
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.
  • Semiconductor Device Technology

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene