Laser-driven detonation wave in hafnium oxide film: Defect controlled laser damage and ablation

Abstract

An ion-beam sputtered film of hafnium oxide was irradiated with an intense nanosecond laser pulse above the ablation threshold. The transmitted laser power was measured as a function of time, with a resolution of a few hundred picoseconds. The spatial origin of the defect-triggered ablation was monitored for each event. A phenomenological model of a rapidly expanding, absorbing disk can explain the observed time dependent transmission and structure sizes of the affected material. The required expansion speeds, ranging from 1 to 100 km/s, and their observed dependence on the local laser intensity, are compatible with a laser-driven detonation wave as described by the Chapman–Jouget (CJ) theory. Because the energy deposited by the laser pulse is too low to explain detonation in a material with the density of hafnium oxide, we hypothesize that the detonation wave propagates in the electron–hole subspace. We modified the CJ theory to describe laser-driven detonation in an electron–hole plasma and to account for plasma expansion sideways to the laser beam.

Document Details

Document Type
Pub Defense Publication
Publication Date
Sep 23, 2020
Source ID
10.1063/5.0015406

Entities

People

  • David H. Dunlap
  • Luke A. Emmert
  • W Rudolph
  • Yejia Xu

Organizations

  • United States Army
  • University of New Mexico

Tags

Fields of Study

  • Physics

Readers

  • Combustion Dynamics and Shock Wave Physics.
  • Pulsed Power and Plasma Physics.
  • Surface Engineering/Surface Coating Technology.

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition
  • Microelectronics
  • Microelectronics - Graphene